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dc.creatorTasić, Gordana
dc.creatorRanđelović, Jelena
dc.creatorVusurović, Nikola
dc.creatorMaslak, Veselin
dc.creatorHusinec, Suren
dc.creatorSavić, Vladimir
dc.date.accessioned2019-09-02T11:34:26Z
dc.date.available2019-09-02T11:34:26Z
dc.date.issued2013
dc.identifier.issn0040-4039
dc.identifier.urihttps://farfar.pharmacy.bg.ac.rs/handle/123456789/1924
dc.description.abstractIntramolecular Pd-catalysed cyclisation reactions for the preparation of bicyclic compounds have been studied as a model system towards the synthesis of corialstonine and corialstonidine. Significant differences in reactivity have been observed for the cyclic allyl alcohols possessing O-protected and free OH functionalities. Cyclisation via the intramolecular Heck reaction, for both derivatives, proved to be highly regioselective and while the O-protected compound favoured the exo mode of cyclisation, the unprotected alcohol preferred the endo cyclisation pathway. Brief computational studies were carried out in order to obtain further insight into these processes.en
dc.publisherPergamon-Elsevier Science Ltd, Oxford
dc.relationinfo:eu-repo/grantAgreement/MESTD/Basic Research (BR or ON)/172009/RS//
dc.rightsrestrictedAccess
dc.sourceTetrahedron-Asymmetry
dc.subjectBicyclic compoundsen
dc.subjectHeck reactionen
dc.subjectRegioselectivityen
dc.subjectCorialstonineen
dc.subjectCorialstonidineen
dc.titleA highly regioselective, protecting group controlled, synthesis of bicyclic compounds via Pd-catalysed intramolecular cyclisationsen
dc.typearticle
dc.rights.licenseARR
dcterms.abstractМаслак, Веселин; Савић, Владимир; Хусинец, Сурен; Ранђеловић, Јелена; Вусуровић, Никола; Тасић, Гордана;
dc.citation.volume54
dc.citation.issue18
dc.citation.spage2243
dc.citation.epage2246
dc.citation.other54(18): 2243-2246
dc.citation.rankM22
dc.identifier.wos000317640800009
dc.identifier.doi10.1016/j.tetlet.2013.02.068
dc.identifier.scopus2-s2.0-84875719109
dc.type.versionpublishedVersion


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