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Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes

Samo za registrovane korisnike
2019
Autori
Petronijević, M.
Agbaba, Jasmina
Ražić, Slavica
Molnar-Jazić, Jelena
Tubić, Aleksandra
Watson, M.
Dalmacija, B.
Članak u časopisu (Objavljena verzija)
Metapodaci
Prikaz svih podataka o dokumentu
Apstrakt
This research evaluates the effect of ultraviolet photolysis, ozonation and ozonation/ultraviolet advanced oxidation processes on different disinfection by-product precursors, during the treatment of water with low organic matter and moderate bromide contents. After different combinations of ultraviolent fluence and ozone, the formation potentials of trihalomethanes and haloacetic acids were investigated. Bromine incorporation factors were used to give specific insight into the behaviour of brominated disinfection by-products, and inorganic bromate formation was also determined. The ozone/ultraviolet process was found to be more effective in reducing the total natural organic matter content than ozonation or ultraviolet photolysis alone. Ultraviolet photolysis was more successful removing the precursors of brominated trihalomethanes than chlorinated trihalomethanes, but slightly increased the precursors of both brominated and chlorinated haloacetic acids. During ozonation, reductions i...n the haloacetic acid formation potential were significantly better than those of the trihalomethanes formation potential (up to 54 and 27%, respectively). In the combined ozonation/ultraviolet process, increasing the ultraviolet fluence had a varying effect on trihalomethane and haloacetic acid precursor behaviour, depending on the ozone dose applied. Bromine incorporation after ozonation alone increased to up to 38% of the total bromide, largely as a result of bromate formation. The combined process curtailed all bromate formation, but increased the bromine incorporation up to 48% at higher ozone doses, with disinfection by-product formation shifting towards the more toxic brominated species.

Ključne reči:
Advanced oxidation processes / Bromine incorporation / Disinfection by-product precursors / Natural organic matter / Ozonation / Ultraviolet photolysis
Izvor:
International Journal of Environmental Science and Technology, 2019, 16, 1, 171-180
Izdavač:
  • Springer, New York
Finansiranje / projekti:
  • Unapređenje remedijacionih tehnologija i razvoj metoda za procenu rizika zagađenih lokaliteta (RS-43005)

DOI: 10.1007/s13762-018-1652-8

ISSN: 1735-1472

WoS: 000455252700015

Scopus: 2-s2.0-85041505308
[ Google Scholar ]
10
8
URI
https://farfar.pharmacy.bg.ac.rs/handle/123456789/3314
Kolekcije
  • Radovi istraživača / Researchers’ publications
Institucija/grupa
Pharmacy
TY  - JOUR
AU  - Petronijević, M.
AU  - Agbaba, Jasmina
AU  - Ražić, Slavica
AU  - Molnar-Jazić, Jelena
AU  - Tubić, Aleksandra
AU  - Watson, M.
AU  - Dalmacija, B.
PY  - 2019
UR  - https://farfar.pharmacy.bg.ac.rs/handle/123456789/3314
AB  - This research evaluates the effect of ultraviolet photolysis, ozonation and ozonation/ultraviolet advanced oxidation processes on different disinfection by-product precursors, during the treatment of water with low organic matter and moderate bromide contents. After different combinations of ultraviolent fluence and ozone, the formation potentials of trihalomethanes and haloacetic acids were investigated. Bromine incorporation factors were used to give specific insight into the behaviour of brominated disinfection by-products, and inorganic bromate formation was also determined. The ozone/ultraviolet process was found to be more effective in reducing the total natural organic matter content than ozonation or ultraviolet photolysis alone. Ultraviolet photolysis was more successful removing the precursors of brominated trihalomethanes than chlorinated trihalomethanes, but slightly increased the precursors of both brominated and chlorinated haloacetic acids. During ozonation, reductions in the haloacetic acid formation potential were significantly better than those of the trihalomethanes formation potential (up to 54 and 27%, respectively). In the combined ozonation/ultraviolet process, increasing the ultraviolet fluence had a varying effect on trihalomethane and haloacetic acid precursor behaviour, depending on the ozone dose applied. Bromine incorporation after ozonation alone increased to up to 38% of the total bromide, largely as a result of bromate formation. The combined process curtailed all bromate formation, but increased the bromine incorporation up to 48% at higher ozone doses, with disinfection by-product formation shifting towards the more toxic brominated species.
PB  - Springer, New York
T2  - International Journal of Environmental Science and Technology
T1  - Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes
VL  - 16
IS  - 1
SP  - 171
EP  - 180
DO  - 10.1007/s13762-018-1652-8
ER  - 
@article{
author = "Petronijević, M. and Agbaba, Jasmina and Ražić, Slavica and Molnar-Jazić, Jelena and Tubić, Aleksandra and Watson, M. and Dalmacija, B.",
year = "2019",
abstract = "This research evaluates the effect of ultraviolet photolysis, ozonation and ozonation/ultraviolet advanced oxidation processes on different disinfection by-product precursors, during the treatment of water with low organic matter and moderate bromide contents. After different combinations of ultraviolent fluence and ozone, the formation potentials of trihalomethanes and haloacetic acids were investigated. Bromine incorporation factors were used to give specific insight into the behaviour of brominated disinfection by-products, and inorganic bromate formation was also determined. The ozone/ultraviolet process was found to be more effective in reducing the total natural organic matter content than ozonation or ultraviolet photolysis alone. Ultraviolet photolysis was more successful removing the precursors of brominated trihalomethanes than chlorinated trihalomethanes, but slightly increased the precursors of both brominated and chlorinated haloacetic acids. During ozonation, reductions in the haloacetic acid formation potential were significantly better than those of the trihalomethanes formation potential (up to 54 and 27%, respectively). In the combined ozonation/ultraviolet process, increasing the ultraviolet fluence had a varying effect on trihalomethane and haloacetic acid precursor behaviour, depending on the ozone dose applied. Bromine incorporation after ozonation alone increased to up to 38% of the total bromide, largely as a result of bromate formation. The combined process curtailed all bromate formation, but increased the bromine incorporation up to 48% at higher ozone doses, with disinfection by-product formation shifting towards the more toxic brominated species.",
publisher = "Springer, New York",
journal = "International Journal of Environmental Science and Technology",
title = "Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes",
volume = "16",
number = "1",
pages = "171-180",
doi = "10.1007/s13762-018-1652-8"
}
Petronijević, M., Agbaba, J., Ražić, S., Molnar-Jazić, J., Tubić, A., Watson, M.,& Dalmacija, B.. (2019). Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes. in International Journal of Environmental Science and Technology
Springer, New York., 16(1), 171-180.
https://doi.org/10.1007/s13762-018-1652-8
Petronijević M, Agbaba J, Ražić S, Molnar-Jazić J, Tubić A, Watson M, Dalmacija B. Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes. in International Journal of Environmental Science and Technology. 2019;16(1):171-180.
doi:10.1007/s13762-018-1652-8 .
Petronijević, M., Agbaba, Jasmina, Ražić, Slavica, Molnar-Jazić, Jelena, Tubić, Aleksandra, Watson, M., Dalmacija, B., "Fate of bromine-containing disinfection by-products precursors during ozone and ultraviolet-based advanced oxidation processes" in International Journal of Environmental Science and Technology, 16, no. 1 (2019):171-180,
https://doi.org/10.1007/s13762-018-1652-8 . .

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