Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices
Само за регистроване кориснике
2023
Аутори
Petronijević, M.Ražić, Slavica
Tubić, A.
Molnar Jazić, J.
Watson, M.
Dalmacija, B.
Agbaba, J.
Чланак у часопису (Објављена верзија)
Метаподаци
Приказ свих података о документуАпстракт
The aim of this study was to investigate the influence of UV/H2O2 advanced oxidation process on the natural organic matter content and disinfection by-products formation potential of different water matrices. Three water matrices (two natural waters and a synthetic humic acid solution) with different natural organic matter characteristics and concentrations were analysed. The carbonaceous disinfection by-products: trihalomethanes, haloacetic acids and haloketones, as well as nitrogenous disinfection by-products: haloacetonitriles and chloropicrin were investigated after chlorination. The UV/H2O2 treatment resulted in significant trihalomethane and haloacetic acids precursors removal (up to 53% and 30%, respectively) in humic acid solution in conditions ≥ 1.0 mg H2O2/mg DOC, in combination with a dose of UV irradiation ≥ 3000 mJ/cm2. Under the same reaction conditions, in natural groundwater rich in hydrophobic natural organic matter, the advanced process was less effective in DBP precu...rsors removal. On the other hand, the advanced process was very effective in trihalomethaneprecursors removal (up to 76%) in groundwater with hydrophyilic natural organic matter. Haloketones were formed after treatment in very low concentrations. Nitrogenous disinfection by-products were only formed in the natural water containing hydrophilic organic matter, during the advanced process at 3.0 mg H2O2/mg DOC. The UV/H2O2 process resulted in negligible organic matter mineralization, but increased the brominated disinfection by-products formation in waters with low to medium bromide contents. It was concluded that under the same advanced oxidation process reaction conditions different natural organic matter structures showed different reactivities with chlorine toward the formation of the investigated disinfection by-products.
Кључне речи:
Advanced oxidation process / Bromine incorporation factor / Disinfection by-products / Natural organic matter / Water treatmentИзвор:
International Journal of Environmental Science and Technology, 2023Издавач:
- Institute for Ionics
Финансирање / пројекти:
- Министарство науке, технолошког развоја и иновација Републике Србије, институционално финансирање - 200134 (Универзитет у Новом Саду, Технолошки факултет) (RS-MESTD-inst-2020-200134)
- Министарство науке, технолошког развоја и иновација Републике Србије, институционално финансирање - 200125 (Универзитет у Новом Саду, Природно-математички факултет) (RS-MESTD-inst-2020-200125)
- Министарство науке, технолошког развоја и иновација Републике Србије, институционално финансирање - 200161 (Универзитет у Београду, Фармацеутски факултет) (RS-MESTD-inst-2020-200161)
DOI: 10.1007/s13762-023-04862-4
ISSN: 1735-1472
WoS: 000946978000002
Scopus: 2-s2.0-85149782752
Институција/група
PharmacyTY - JOUR AU - Petronijević, M. AU - Ražić, Slavica AU - Tubić, A. AU - Molnar Jazić, J. AU - Watson, M. AU - Dalmacija, B. AU - Agbaba, J. PY - 2023 UR - https://farfar.pharmacy.bg.ac.rs/handle/123456789/4552 AB - The aim of this study was to investigate the influence of UV/H2O2 advanced oxidation process on the natural organic matter content and disinfection by-products formation potential of different water matrices. Three water matrices (two natural waters and a synthetic humic acid solution) with different natural organic matter characteristics and concentrations were analysed. The carbonaceous disinfection by-products: trihalomethanes, haloacetic acids and haloketones, as well as nitrogenous disinfection by-products: haloacetonitriles and chloropicrin were investigated after chlorination. The UV/H2O2 treatment resulted in significant trihalomethane and haloacetic acids precursors removal (up to 53% and 30%, respectively) in humic acid solution in conditions ≥ 1.0 mg H2O2/mg DOC, in combination with a dose of UV irradiation ≥ 3000 mJ/cm2. Under the same reaction conditions, in natural groundwater rich in hydrophobic natural organic matter, the advanced process was less effective in DBP precursors removal. On the other hand, the advanced process was very effective in trihalomethaneprecursors removal (up to 76%) in groundwater with hydrophyilic natural organic matter. Haloketones were formed after treatment in very low concentrations. Nitrogenous disinfection by-products were only formed in the natural water containing hydrophilic organic matter, during the advanced process at 3.0 mg H2O2/mg DOC. The UV/H2O2 process resulted in negligible organic matter mineralization, but increased the brominated disinfection by-products formation in waters with low to medium bromide contents. It was concluded that under the same advanced oxidation process reaction conditions different natural organic matter structures showed different reactivities with chlorine toward the formation of the investigated disinfection by-products. PB - Institute for Ionics T2 - International Journal of Environmental Science and Technology T1 - Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices DO - 10.1007/s13762-023-04862-4 ER -
@article{ author = "Petronijević, M. and Ražić, Slavica and Tubić, A. and Molnar Jazić, J. and Watson, M. and Dalmacija, B. and Agbaba, J.", year = "2023", abstract = "The aim of this study was to investigate the influence of UV/H2O2 advanced oxidation process on the natural organic matter content and disinfection by-products formation potential of different water matrices. Three water matrices (two natural waters and a synthetic humic acid solution) with different natural organic matter characteristics and concentrations were analysed. The carbonaceous disinfection by-products: trihalomethanes, haloacetic acids and haloketones, as well as nitrogenous disinfection by-products: haloacetonitriles and chloropicrin were investigated after chlorination. The UV/H2O2 treatment resulted in significant trihalomethane and haloacetic acids precursors removal (up to 53% and 30%, respectively) in humic acid solution in conditions ≥ 1.0 mg H2O2/mg DOC, in combination with a dose of UV irradiation ≥ 3000 mJ/cm2. Under the same reaction conditions, in natural groundwater rich in hydrophobic natural organic matter, the advanced process was less effective in DBP precursors removal. On the other hand, the advanced process was very effective in trihalomethaneprecursors removal (up to 76%) in groundwater with hydrophyilic natural organic matter. Haloketones were formed after treatment in very low concentrations. Nitrogenous disinfection by-products were only formed in the natural water containing hydrophilic organic matter, during the advanced process at 3.0 mg H2O2/mg DOC. The UV/H2O2 process resulted in negligible organic matter mineralization, but increased the brominated disinfection by-products formation in waters with low to medium bromide contents. It was concluded that under the same advanced oxidation process reaction conditions different natural organic matter structures showed different reactivities with chlorine toward the formation of the investigated disinfection by-products.", publisher = "Institute for Ionics", journal = "International Journal of Environmental Science and Technology", title = "Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices", doi = "10.1007/s13762-023-04862-4" }
Petronijević, M., Ražić, S., Tubić, A., Molnar Jazić, J., Watson, M., Dalmacija, B.,& Agbaba, J.. (2023). Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices. in International Journal of Environmental Science and Technology Institute for Ionics.. https://doi.org/10.1007/s13762-023-04862-4
Petronijević M, Ražić S, Tubić A, Molnar Jazić J, Watson M, Dalmacija B, Agbaba J. Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices. in International Journal of Environmental Science and Technology. 2023;. doi:10.1007/s13762-023-04862-4 .
Petronijević, M., Ražić, Slavica, Tubić, A., Molnar Jazić, J., Watson, M., Dalmacija, B., Agbaba, J., "Influence of UV/H2O2 processes on C- and N-disinfection by-products formation in different water matrices" in International Journal of Environmental Science and Technology (2023), https://doi.org/10.1007/s13762-023-04862-4 . .